I'm a statistician so I could just tell you the answer? But I think showing you how to get it might serve you better as a game designer. What you are attempting to do is just a series of binomials. Excel can actually do this for you quite easily:
http://www.ehow.com/how_8231796_use-excel-binomial-probability.html
The basic argument is = 1-BINOMDIST(1,X,0.166666667,TRUE)
This gives you two or more successes. Replace X with your dice pool of 5, 6, etc. If you want three or more successes then change the 1 before the X to 2.
If you don't have excel, here's an online binomial calculator I can walk you through.
http://stattrek.com/online-calculator/binomial.aspx
The probability on a single success is 1/6 or roughly .1666667.
The number of trials is your dice pool size.
The number of successes in your given example is 2.
The probability that you're looking for is "Cumulative Probability: P(X > 2)"
To find the probability for 3 or more successes, just change the number of successes to 3.
Edit: Added more information and clarified the Excel syntax.