Be polite and address the behavior, not the person. Remember that if the conversation is longer than two words ("**** off") the goal of the conversation is to maintain the relationship by preventing the problem behavior from destroying it. The problem behavior isn't their fault, it's just something that they need to stop doing in your presence.
"Man, I like you and I love having you in our game, but this thing is ruining the game for everyone."
Treat it like you're taking away a homebrew magical item you accidentally made too powerful. It's not bad and it's not their fault (even if it really, really is), it's just a problem that you need their help fixing. Your goal is not to get them to apologize for their behavior, it's to convince them to agree to something–and keep the agreement–so that you can thank them for it. And when that conversation is over, you're back to the two word response: either "**** off" or "thank you".